Keywords
thermal spray, aluminum, HDPE, electrical conductivity, Taguchi methodology
Document Type
Research Paper
Abstract
Metallization involves applying a thin metal layer onto a substrate, typically through techniques such as thermal spraying. This process improves conductivity, durability, and aesthetic appeal, making it valuable in applications such as electronics, solar panels, and decorative coatings. In this study, flame thermal spray technique are used to metalize high-density polyethylene with an aluminum layer. Taguchi and ANOVA are used to investigate the effect of various parameters on the adhesion strength between aluminum layers deposited on high-density polyethylene (HDPE) substrates. DOE utilization has facilitated the identification of the effects of the flame thermal spraying parameters, such as the distance between the spray gun and substrate, the spray velocity, the powder feed rate, and the delay time, on the adhesion strength. The orthogonal matrix resulting from the Taguchi method corresponded to an L9 (34) matrix, which was utilized to decrease the number of experiments from 81 to 9. To attain optimal adhesion strength, it is essential to maintain a distance of 250 mm between the gun spray and the substrate, utilize a powder feeding rate of 15 g/minute, achieve a spraying velocity of 300 m/min, and implement a delay time of four minutes. The X-ray diffraction shows that there is no oxidation in the coating layer. Moreover, the aluminum layer shows good electrical conductivity (2.08×104 Ω-1.cm-1). Using Taguchi and ANOVA leads to optimizing processes efficiently with fewer trials, improving product quality by reducing variability, and making informed decisions on which factors to control for optimal performance.
References
J. T. Tsai, S. Akin, D. F. Bahr, and M. B.-G. Jun, A predictive modeling approach for cold spray metallization on polymers, Surf. Coat. Technol., 483 (2024) 130711. https://doi.org/10.1016/j.surfcoat.2024.130711 A. Zhang, W. Wu, and D. Xie, Influence of laser treatment on the adhesion force of metallized carbon fiber reinforced polymer (CFRP) composite, Int. J. Adhes. Adhes., 135 (2024) 103830. https://doi.org/10.1016/j.ijadhadh.2024.103830 H. Zhang, R. Xu, and T. Zhou, Selective Metallization of Thermoplastic Elastomers Based on Laser‐Induced Surface Activation, Adv. Eng. Mater., 26 (2024) 2301715. https://doi.org/10.1002/adem.202301715 Q. Duan and Y. Lu, Metallized liquid crystal polymer with low interfacial roughness and excellent adhesive strength based on semi-additive process for high-frequency signal transmission, Appl. Surf. Sci., 649 (2024) 159144. https://doi.org/10.1016/j.apsusc.2023.159144 R. Melentiev, A. Yudhanto, R. Tao, T. Vuchkov, and G. Lubineau, Metallization of polymers and composites: State-of-the-art approaches, Mater. Des., 221 (2022) 110958. https://doi.org/10.1016/j.matdes.2022.110958 F. Faupel, T. Strunskus, M. Kiene, A. Thran, C. Bechtolsheim, and V. Zaporojtchenko, Fundamental aspects of polymer metallization, MRS Online Proc. Lib., 511 (1998) 15-26. https://doi.org/10.1557/PROC-511-15 Chiu, P. G., and D.T. Hsu, H.K. Kim, F.G. Shi, H.S. Nalwa. 2001. Chapter 6 - Low-k materials for microelectronics interconnects, In Handbook of Advanced Electronic and Photonic Materials and Devices, Vol. 4, pp. 201-234. Academic Press. https://doi.org/10.1016/B978-012513745-4/50041-X G. J. Matrood, A. M. Al-Gaban, and H. M. Yousif, Studying the Erosion Corrosion Behavior of NiCrAlY Coating Layer Applied on AISI 446 Stainless Steel Using Thermal Spray Technique, Eng. Technol. J., 38 (2020) 1676-1683. https://doi.org/10.30684/etj.v38i11A.1691 P. Fauchais, G. Montavon, and G. Bertrand, From powders to thermally sprayed coatings, J. Therm. Spray Technol., 19 (2010) 56-80. https://doi.org/10.1007/s11666-009-9435-x V. Lakkannavar, K. Yogesha, C. D. Prasad, R. K. Phanden, G. Srinivasa, and S. C. Prasad, Thermal spray coatings on high-temperature oxidation and corrosion applications–a comprehensive review, Results Surf. Interfaces, 16 (2024) 100250. https://doi.org/10.1016/j.rsurfi.2024.100250 G. M. Whitesides, Nanoscience, nanotechnology, and chemistry, Small, 1 (2005) 172-179. https://doi.org/10.1002/smll.200400130 .H. A. Akkar and S. Khalooq, Characteristics and evaluation of nano electronic devices, Eng. Technol. J., 32 (2014) 486-497. https://doi.org/10.30684/etj.32.3B.10 D. R. Baer, J. E. Amonette, M. H. Engelhard, D. J. Gaspar, A. S. Karakoti, S. Kuchibhatla, and C. M. Wang, Characterization challenges for nanomaterials, Surf. Interface Anal., 40 (2008) 529-537. https://doi.org/10.1002/sia.2726 T. A. Saleh, Properties of nanoadsorbents and adsorption mechanisms, Interface Sci. Technol., 34 (2022) 233-263. https://doi.org/10.1016/B978-0-12-849876-7.00010-5 J. Meziani, C. E. Bunker, F. Lu, H. Li, W. Wang, E. A. Guliants, & Y. P. Sun, , Formation and properties of stabilized aluminum nanoparticles, ACS Appl. Mater. Interfaces, 1 (2009) 703-709. https://doi.org/10.1021/am800209m B. Medasani and I. Vasiliev, Computational study of the surface properties of aluminum nanoparticles, Surf. Sci., 603 (2009) 2042-2046. https://doi.org/10.1016/j.susc.2009.03.025 B. Reeja‐Jayan, P. Kovacik, R. Yang, A route towards sustainability through engineered polymeric interfaces, Adv. Mater. Interfaces, 1 (2014) 1400117. https://doi.org/10.1002/admi.201400117 S. R. Jalal, Comparison OF Shear Properties for High Density Polyethylene (HDPE) and Poly vinyl Cloride (PVC) Polymers, Eng Technol. J., 33 (2015) 2039-2048. https://doi.org/10.30684/etj.2015.116222 R.K. Roy, Design of Experiments Using Taguchi Approach: 16 Steps to Product and Process Improvement, Wiley, Hoboken, 2001, https://doi.org/10.1520/JTE12406JISBN 0-471-36101-1 T. Ermergen and F. Taylan, Investigation of DOE model analyses for open atmosphere laser polishing of additively manufactured Ti-6Al-4V samples by using ANOVA, Opt. Laser Technol., 168 (2024) 109832. https://doi.org/10.1016/j.optlastec.2023.109832 S.K. Madhavi, D. Sreeramulu, and M. Venkatesh, Evaluation of Optimum Turning Process of Process Parameters Using DOE andPCA Taguchi Method, Mater. Today, Proc., 4 (2017) 1937-1946. https://doi.org/10.1016/j.matpr.2017.02.039 H.V. Pham, H.P. Nguyen, S. Shailesh, D.T. Nguyen, N.T. Bui, Investigating Technological Parameters and TiN-Coated Electrodes for Enhanced Efficiency in Ti-6Al-4V Micro-EDM Machining, Metals, 14 (2024) 1-13. https://doi.org/10.3390/met14020162 B. Yelamasetti, M. Sandeep, S. Narella, V. Tiruchanur, T. Sonar, C. Prakash, & S. Kumar, Optimization of TIG welding process parameters using Taguchi technique for the joining of dissimilar metals of AA5083 and AA7075, Sci. Rep., 14 (2024) 23694. https://doi.org/10.1038/s41598-024-74458-6 H. L. Alwan, B. M. Albaghdadi, M. M. AL-Khafaji, and A. A. Abbas, Estimation of cutting tool wear in turning using Taguchi method depending on weight of the removed tool metal, Eng. Technol. J., 32 (2014) 24-33. https://doi.org/10.30684/etj.32.1A.3 J. Lu, L. Ni, S. Wang, and X. Mao, Grey-Taguchi analysis and experimental assessment of 1 GPa HSLA steel treated by quenching and tempering, J. Mater. Res. Technol., 29 (2024) 3508-3521. https://doi.org/10.1016/j.jmrt.2024.02.100 S. Kulkarni and J. V. Gohel, Enhanced performance of perovskite solar cell by optimization of thin film control parameters using Taguchi method, Optik, p. 172090, 2024. https://doi.org/10.1016/j.ijleo.2024.172090 J. Voyer, P. Schulz, and M. Schreiber, Electrically conductive flame sprayed aluminum coatings on textile substrates, J. Therm. Spray Technol., 17 (2008) 818-823. https://doi.org/10.1007/s11666-008-9228-7 H. Ashrafizadeh, P. Mertiny, A. McDonald, Evaluation of the Influence of Flame Spraying Parameters on Microstructure and Electrical Conductivity of Al-12Si Coatings Deposited on Polyurethane Substrates, International Thermal Spray Conference, ASM International, 2015, 370-376. https://doi.org/10.31399/asm.cp.itsc2015p0370 N. Huonnic, M. Abdelghani, P. Mertiny, and A. McDonald, Deposition and characterization of flame-sprayed aluminum on cured glass and basalt fiber-reinforced epoxy tubes, Surf. Coat. Technol., 205 (2010) 867-873. https://doi.org/10.1016/j.surfcoat.2010.08.029 J. Affi, H. Okazaki, M. Yamada, and M. Fukumoto, Fabrication of aluminum coating onto CFRP substrate by cold spray, Mater. Trans., 52 (2011) 1759-1763. https://doi.org/10.2320/matertrans.T-M2011807 A. J. Mohammed, H. A. Yousif, and S. S. Ahmed, Improving the deposition efficiency of the flame thermal spray coating process using ANOVA, in AIP Conf. Proc., 3105 (2024) AIP Publishing. https://doi.org/10.1063/5.0213307 G. J. Matrood, N. J. Abdulkader, N. M. Ali, N.M., Study of behaviour and morphology of corrosion region of copper layer coated on polymer substrates by flame thermal spraying, International Information and Engineering Technology Association, Revue des Composites et des Matériaux Avancés-Journal of Composite and Advanced Materials, 34 (2024) 653-660. https://doi.org/10.18280/rcma.340513 F. H. Edan, Prediction of Contact Angle for Sintered Alloy for Solid Freeform Fabrication, Eng Technol. J., 34 (2016) 1666-1672. http://dx.doi.org/10.30684/etj.34.8A.16 N. X. Randall, The current state-of-the-art in scratch testing of coated systems, Surf. Coat. Technol., 380 (2019) 125092. https://doi.org/10.1016/j.surfcoat.2019.125092 J. Li and W. Beres, Scratch test for coating/substrate systems–A literature review, Can. Metall. Q., 46 (2007) 155-173 https://doi.org/10.1179/cmq.2007.46.2.155 S. Bull and E. Berasetegui, An overview of the potential of quantitative coating adhesion measurement by scratch testing, Tribol. Int., 39 (2006) 99-114. https://doi.org/10.1016/j.triboint.2005.04.013 M. Kalin and M. Polajnar, The correlation between the surface energy, the contact angle and the spreading parameter, and their relevance for the wetting behaviour of DLC with lubricating oils, Tribol. Int., 66 (2013) 225-233. https://doi.org/10.1016/j.triboint.2013.05.007 A. A. AbdulRazak, Z. M. Shakor, and S. Rohani, Optimizing Biebrich Scarlet removal from water by magnetic zeolite 13X using response surface method, J. Environ. Chem. Eng., 6 (2018) 6175-6183. https://doi.org/10.1016/j.jece.2018.09.043 L. Moraga, R. Henriquez, and B. Solis, Quantum theory of the effect of grain boundaries on the electrical conductivity of thin films and wires, Physica B: Condensed Matter, 470 (2015) 39-49. https://doi.org/10.1016/j.physb.2015.04.034
Highlights
Metallic coatings on HDPE substrates were studied using the flame thermal spray technique. The effect of thermal spray parameters on adhesion strength was investigated. Metallic powder enabled successful coating without damaging the polymeric substrate.
Recommended Citation
Matrood, Ghufran; Abdulkader, Niveen; and Ali, Nahedh
(2024)
"Investigating the effect of spray parameters on adhesion strength between aluminum coatings and polymeric substrate,"
Engineering and Technology Journal: Vol. 42:
Iss.
12, Article 5.
DOI: https://doi.org/10.30684/etj.2024.155226.1850
DOI
10.30684/etj.2024.155226.1850
First Page
1484
Last Page
1494





